Single-photon superradiance in individual caesium lead halide quantum dots

Single-photon superradiance in individual caesium lead halide quantum dots

31 January 2024 | Chenglian Zhu1,2, Simon C. Boehme1,2, Leon G. Feld1,2, Anastasiiia Moskalenko1,2, Dmitry N. Dirin1,2, Rainer F. Mahrt3, Thilo Stöferle3, Maryna I. Bodnarchuk1,2, Alexander L. Efros4, Peter C. Sercel5,6, Maksym V. Kovalenko1,2,7,8,9 and Gabriele Rainò1,2,9
The study investigates single-photon superradiance in individual CsPbX₃ (X = Cl, Br, I) perovskite quantum dots (QDs), achieving sub-100 ps radiative decay times, comparable to the reported exciton coherence time. The findings suggest the formation of giant transition dipoles, confirmed by effective-mass calculations. The results highlight the potential for ultrabright, coherent quantum light sources and demonstrate that quantum effects, such as single-photon emission, persist in nanoparticles ten times larger than the exciton Bohr radius. The research also explores the size-, temperature-, and composition-dependent radiative lifetimes, providing a comprehensive understanding of the cooperative emission process. The findings contribute to the development of scalable and integrable material platforms for quantum applications.The study investigates single-photon superradiance in individual CsPbX₃ (X = Cl, Br, I) perovskite quantum dots (QDs), achieving sub-100 ps radiative decay times, comparable to the reported exciton coherence time. The findings suggest the formation of giant transition dipoles, confirmed by effective-mass calculations. The results highlight the potential for ultrabright, coherent quantum light sources and demonstrate that quantum effects, such as single-photon emission, persist in nanoparticles ten times larger than the exciton Bohr radius. The research also explores the size-, temperature-, and composition-dependent radiative lifetimes, providing a comprehensive understanding of the cooperative emission process. The findings contribute to the development of scalable and integrable material platforms for quantum applications.
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[slides and audio] Single-photon superradiance in individual caesium lead halide quantum dots