Time-resolved atomic inner-shell spectroscopy

Time-resolved atomic inner-shell spectroscopy

24 OCTOBER 2002 | M. Drescher*,†, M. Hentschel*, R. Kienberger*, M. Uiberacker*, V. Yakovlev*, A. Scrinzi*, Th. Westerwalbesloh†, U. Kleineberg†, U. Heinzmann† & F. Krausz*
The paper presents a novel approach to time-resolved atomic inner-shell spectroscopy using a laser-based sampling system. This system, consisting of a few-femtosecond visible light pulse and a synchronized sub-femtosecond soft X-ray pulse, allows for direct observation of the relaxation dynamics of core-excited atoms in the time domain with attosecond resolution. The authors measured the lifetime of M-shell vacancies in krypton, finding a value of 7.9 ± 1.0 fs. The technique is based on the creation of a core hole by exciting an electron from an inner shell and the subsequent decay of this hole, which is probed using a delayed visible light pulse. The study demonstrates the feasibility of attosecond atomic spectroscopy and opens new avenues for understanding the dynamics of multi-electron systems in strong fields.The paper presents a novel approach to time-resolved atomic inner-shell spectroscopy using a laser-based sampling system. This system, consisting of a few-femtosecond visible light pulse and a synchronized sub-femtosecond soft X-ray pulse, allows for direct observation of the relaxation dynamics of core-excited atoms in the time domain with attosecond resolution. The authors measured the lifetime of M-shell vacancies in krypton, finding a value of 7.9 ± 1.0 fs. The technique is based on the creation of a core hole by exciting an electron from an inner shell and the subsequent decay of this hole, which is probed using a delayed visible light pulse. The study demonstrates the feasibility of attosecond atomic spectroscopy and opens new avenues for understanding the dynamics of multi-electron systems in strong fields.
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